We present an extended x-ray absorption fine structure study of the pyrochlore Y2Ru2O7 (8-298 K). We find evidence, on a local scale, of a significant magnetoelastic coupling at the Neel temperature T-N similar to 77 K pointed out by a huge Debye-Waller sigma(2) factor deviation from a correlated temperature dependent Debye-like local order behavior plus a temperature independent static contribution. Moreover, we notice the occurrence of a potential local order-disorder structural phase transition at T* = 150 K. This anomalous behavior is consistent with the pyrochlore's predisposition towards structural disorder and with a strong spin-phonon correlation. Remarkably the low-temperature order competes with the tendency of magnetic frustration to induce a less symmetric local structure.

Evidence of local structural order and spin-lattice coupling in the frustrated pyrochlore Y2Ru2 O7

SANNA, SAMUELE;CARRETTA, PIETRO;
2015-01-01

Abstract

We present an extended x-ray absorption fine structure study of the pyrochlore Y2Ru2O7 (8-298 K). We find evidence, on a local scale, of a significant magnetoelastic coupling at the Neel temperature T-N similar to 77 K pointed out by a huge Debye-Waller sigma(2) factor deviation from a correlated temperature dependent Debye-like local order behavior plus a temperature independent static contribution. Moreover, we notice the occurrence of a potential local order-disorder structural phase transition at T* = 150 K. This anomalous behavior is consistent with the pyrochlore's predisposition towards structural disorder and with a strong spin-phonon correlation. Remarkably the low-temperature order competes with the tendency of magnetic frustration to induce a less symmetric local structure.
2015
Applied Physics/Condensed Matter/Materials Science encompasses the resources of three related disciplines: Applied Physics, Condensed Matter Physics, and Materials Science. The applied physics resources are concerned with the applications of topics in condensed matter as well as optics, vacuum science, lasers, electronics, cryogenics, magnets and magnetism, acoustical physics and mechanics. The condensed matter physics resources are concerned with the study of the structure and the thermal, mechanical, electrical, magnetic and optical properties of condensed matter. They include superconductivity, surfaces, interfaces, thin films, dielectrics, ferroelectrics and semiconductors. The materials science resources are concerned with the physics and chemistry of materials and include ceramics, composites, alloys, metals and metallurgy, nanotechnology, nuclear materials, adhesion and adhesives. Resources dealing with polymeric materials are listed in the Organic Chemistry/Polymer Science category.
Esperti anonimi
Inglese
Internazionale
STAMPA
91
22
224101
x-ray absorption, frustrated magnetism
http://harvest.aps.org/bagit/articles/10.1103/PhysRevB.91.224101/apsxml
10
info:eu-repo/semantics/article
262
Castellano, C; Berti, G.; Sanna, Samuele; Ruiz Bustos, R.; Van Duijn, J.; Brambilla, A.; Muñoz Noval, Á.; Carretta, Pietro; Duò, L.; Demartin, F....espandi
1 Contributo su Rivista::1.1 Articolo in rivista
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11571/1179926
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