The nonlinear absorption of Au-Ag nanoplanets made by Ar irradiation of bimetallic nanoclusters in silica has been experimentally investigated by means of the single beam z-scan technique. The measurements have been performed in the picoseconds regime in order to isolate the fast electronic contribution to the third-order nonlinearity. The results reveal large nonlinear absorption properties of these systems, characterized by the concomitance of saturable and reverse saturable absorption. A phenomenological expression has been developed to fit the z-scan curves and to quantitatively determine the nonlinear optical parameters. © 2010 Elsevier B.V. All rights reserved.
Nonlinear optical properties of Au-Ag nanoplanets made by ion beam processing of bimetallic nanoclusters in silica
Pellegrini G.;
2010-01-01
Abstract
The nonlinear absorption of Au-Ag nanoplanets made by Ar irradiation of bimetallic nanoclusters in silica has been experimentally investigated by means of the single beam z-scan technique. The measurements have been performed in the picoseconds regime in order to isolate the fast electronic contribution to the third-order nonlinearity. The results reveal large nonlinear absorption properties of these systems, characterized by the concomitance of saturable and reverse saturable absorption. A phenomenological expression has been developed to fit the z-scan curves and to quantitatively determine the nonlinear optical parameters. © 2010 Elsevier B.V. All rights reserved.I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.