In this work sharp silver nanotips are analyzed and proposed as useful plasmonic tools to reduce the threshold for the onset of strong coupling in the electromagnetic interaction of a point-like emitter with localized surface plasmons. If compared to similarly-sized spherical nanoparticles, conically-shaped nanoparticles turn out to be extremely useful to reduce the oscillator strength requirements for the emitting dipole, a reduction of the threshold by one sixth being obtained in a double cone configuration. Moreover the transition to the strong coupling regime is analyzed for several cone apertures, revealing a nonmonotonic behavior with the appearance of an optimal cone geometry. The emitted-light spectrum is obtained from the computation of the perturbative decay rate and photonic Lamb shift in the classical framework of the Discrete Dipole Approximation. This combined classical-quantum electrodynamics treatment is useful for the theoretical investigation on nonperturbative light-matter interactions involving complex shaped nanoparticles or aggregates.

Strong coupling between a dipole emitter and localized plasmons: enhancement by sharp silver tips

D'AGOSTINO, STEFANIA;ALPEGGIANI, FILIPPO;ANDREANI, LUCIO
2013-01-01

Abstract

In this work sharp silver nanotips are analyzed and proposed as useful plasmonic tools to reduce the threshold for the onset of strong coupling in the electromagnetic interaction of a point-like emitter with localized surface plasmons. If compared to similarly-sized spherical nanoparticles, conically-shaped nanoparticles turn out to be extremely useful to reduce the oscillator strength requirements for the emitting dipole, a reduction of the threshold by one sixth being obtained in a double cone configuration. Moreover the transition to the strong coupling regime is analyzed for several cone apertures, revealing a nonmonotonic behavior with the appearance of an optimal cone geometry. The emitted-light spectrum is obtained from the computation of the perturbative decay rate and photonic Lamb shift in the classical framework of the Discrete Dipole Approximation. This combined classical-quantum electrodynamics treatment is useful for the theoretical investigation on nonperturbative light-matter interactions involving complex shaped nanoparticles or aggregates.
2013
The Physics category includes resources of a broad, general nature that contain materials from all areas of physics, The category also includes resources specifically concerned with the following physics sub-fields: mathematical physics, particle and nuclear physics, physics of fluids and plasmas, quantum physics, and theoretical physics.
Esperti anonimi
Inglese
Internazionale
ELETTRONICO
21
23
27602
27610
9
The journal is among the most widespread ones in Optics.
Strong coupling; light-matter interaction; metal nanoantennas
http://www.opticsinfobase.org/oe/abstract.cfm?uri=oe-21-23-27602
3
info:eu-repo/semantics/article
262
D'Agostino, Stefania; Alpeggiani, Filippo; Andreani, Lucio
1 Contributo su Rivista::1.1 Articolo in rivista
none
File in questo prodotto:
Non ci sono file associati a questo prodotto.

I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.

Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11571/763231
Citazioni
  • ???jsp.display-item.citation.pmc??? ND
  • Scopus 29
  • ???jsp.display-item.citation.isi??? 29
social impact